| Oriented structural design of MXene electrodes for lithium sulfur catalysis | |
| Wang, Yu1,3; Li, Jiaming3; Gu, Qinhua2,6; Liu, Zhilin7; Zhang, Hengrui3; Zheng, Shunri3; Xu, Shichong3; Tan, Kar Ban4; Luo, Yaxiao1; Yu, Zhaoliang3; Li, Haibo3,5; Han, Wenjuan3; Zhang, Mingzhe1; Lu, Ming3; Zhang, Bingsen2,6 | |
| 通讯作者 | Han, Wenjuan(hanwj@jlnu.edu.cn) ; Zhang, Mingzhe(zhangmz@jlu.edu.cn) ; Lu, Ming(luming@jlnu.edu.cn) ; Zhang, Bingsen(bszhang@imr.ac.cn) |
| 2024-12-01 | |
| 发表期刊 | JOURNAL OF ENERGY CHEMISTRY
 |
| ISSN | 2095-4956 |
| 卷号 | 99页码:66-73 |
| 摘要 | The lithium-sulfur reaction can contribute to the chemical electrical energy conversion capacity due to the multi-level ion/electron transfer process. However, the appearance of soluble intermediate products prevents efficient electron transfer, making it impossible to achieve stable cycling and capacity contribution. Restricted catalysis provides a solution for inhibiting the shuttle of soluble lithium polysulfides. Herein, MXene aerogel with optimized channel utilization is designed as S host according to the polysulfide control strategy of localization, adsorption, and catalysis. With the help of the results of oriented channels, the polysulfide conversion process is optimized, providing a comprehensive scheme for inhibiting the shuttle effect. Lithium sulfur catalytic batteries have achieved high capacity and stable cycling. This system provides a comprehensive solution for lithium sulfur reaction catalysis and a new perspective for the functional application of MXene based lithium sulfur batteries. (c) 2024 Science Press and Dalian Institute of Chemical Physics, Chinese Academy of Sciences. Published by ELSEVIER B.V. and Science Press. All rights are reserved, including those for text and data mining, AI training, and similar technologies. |
| 关键词 | MXene Aerogel Lithium-sulfur battery Catalyst |
| 资助者 | Development Plan of Science and Technology of Jilin Province, China ; Natural Science Foundation of Jilin Province ; Innovation Laboratory Development Program of Education Department of Jilin Province ; Industry and Information Technology Department of Jilin Province, China ; MXene Research Support Plan of Jilin 11 Technology Co., Ltd. China |
| DOI | 10.1016/j.jechem.2024.07.038 |
| 收录类别 | SCI |
| 语种 | 英语 |
| 资助项目 | Development Plan of Science and Technology of Jilin Province, China[YDZJ202301ZYTS280] ; Natural Science Foundation of Jilin Province[YDZJ202401316ZYTS] ; Innovation Laboratory Development Program of Education Department of Jilin Province ; Industry and Information Technology Department of Jilin Province, China ; MXene Research Support Plan of Jilin 11 Technology Co., Ltd. China |
| WOS研究方向 | Chemistry ; Energy & Fuels ; Engineering |
| WOS类目 | Chemistry, Applied ; Chemistry, Physical ; Energy & Fuels ; Engineering, Chemical |
| WOS记录号 | WOS:001290172700001 |
| 出版者 | ELSEVIER |
| 引用统计 | |
| 文献类型 | 期刊论文 |
| 条目标识符 | http://ir.imr.ac.cn/handle/321006/188864 |
| 专题 | 中国科学院金属研究所 |
| 通讯作者 | Han, Wenjuan; Zhang, Mingzhe; Lu, Ming; Zhang, Bingsen |
| 作者单位 | 1.Jilin Univ, Coll Phys, State Key Lab Superhard Mat, Changchun 130012, Jilin, Peoples R China 2.Chinese Acad Sci, Inst Met Res, Shenyang Natl Lab Mat Sci, Shenyang 110016, Liaoning, Peoples R China 3.Jilin Normal Univ, Key Lab Funct Mat Phys & Chem, Joint Lab MXene Mat, Minist Educ, Changchun 130103, Jilin, Peoples R China 4.Univ Putra Malaysia, Fac Sci, Dept Chem, Serdang 43400, Selangor, Malaysia 5.Changchun Coll Elect Technol, Sch Optoelect Sci, Changchun 130114, Jilin, Peoples R China 6.Univ Sci & Technol China, Sch Mat Sci & Engn, Shenyang 110016, Liaoning, Peoples R China 7.Shanghai Jiao Tong Univ, Frontiers Sci Ctr Transformat Mol, Sch Chem & Chem Engn, Shanghai 200240, Peoples R China |
| 推荐引用方式 GB/T 7714 | Wang, Yu,Li, Jiaming,Gu, Qinhua,et al. Oriented structural design of MXene electrodes for lithium sulfur catalysis[J]. JOURNAL OF ENERGY CHEMISTRY,2024,99:66-73. |
| APA | Wang, Yu.,Li, Jiaming.,Gu, Qinhua.,Liu, Zhilin.,Zhang, Hengrui.,...&Zhang, Bingsen.(2024).Oriented structural design of MXene electrodes for lithium sulfur catalysis.JOURNAL OF ENERGY CHEMISTRY,99,66-73. |
| MLA | Wang, Yu,et al."Oriented structural design of MXene electrodes for lithium sulfur catalysis".JOURNAL OF ENERGY CHEMISTRY 99(2024):66-73. |
| 条目包含的文件 | 条目无相关文件。 | |||||
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