Mesoporous Pt/N-TiO2/Ti Photocatalytic Plate for Highly Efficient Hydrogen Production | |
Hua, Zhe1,2; Yang, Liu3; Li, Jing1,2; Wang, Junchao3; Chen, Lixin1,2; Tan, Liyuan1,2; Guo, Jiaming1,2; Yao, Jinlei4; Liu, Baodan1,2 | |
通讯作者 | Li, Jing(lijing1@mail.neu.edu.cn) ; Yao, Jinlei(jlyao@usts.edu.cn) ; Liu, Baodan(liubaodan@mail.neu.edu.cn) |
2024-05-25 | |
发表期刊 | CHEMCATCHEM
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ISSN | 1867-3880 |
页码 | 10 |
摘要 | Monolithic plate-type photocatalyst with excellent light absorption, abundant active sites and strong mechanical adhesion is the growing trend of photocatalysis application, as referring to a photovoltaic panel. In this study, we report a large-scale Pt/N-TiO2/Ti photocatalytic plate with granular and mesoporous structure, which shows a superior photocatalytic performance and adhesion than nanowires and nanosheets photocatalysts. The outstanding photocatalytic performance of Pt/N-TiO2/Ti is attributed to the large exposed surface area, enhanced light absorption, high separation efficiency of photogenerated carriers and excellent surface activity induced by single Pt atom cocatalyst. The best Pt/N-TiO2/Ti sample could exhibit an outstanding photocatalytic hydrogen production activity of 72547.9 mu mol & sdot; h(-1) & sdot; g(-1), and a high apparent quantum efficiency of 47.07 % under a 350 nm light irradiation. It can be anticipated that the proposed method and insights would pave a solid way on the development and application of superior TiO2 based photocatalytic plate. |
关键词 | H-2 N doping photocatalyst TiO2 water splitting |
资助者 | National Natural Science Foundation of China ; Guangdong Basic and Applied Basic Research Foundation ; Fundamental Research Funds for the Central Universities ; Development Start-up Foundation of Foshan Graduate School of Innovation, Northeastern University ; Scientific Research Project of Foshan Talents ; Open Fund of the State Key Laboratory of Optoelectronic Materials and Technologies (Sun Yat-Sen University) |
DOI | 10.1002/cctc.202400398 |
收录类别 | SCI |
语种 | 英语 |
资助项目 | National Natural Science Foundation of China ; Guangdong Basic and Applied Basic Research Foundation[2022 A1515011170] ; Guangdong Basic and Applied Basic Research Foundation[2023 A1515010678] ; Fundamental Research Funds for the Central Universities[N2229002] ; Fundamental Research Funds for the Central Universities[N2429001] ; Development Start-up Foundation of Foshan Graduate School of Innovation, Northeastern University[FSNEU20201016001] ; Development Start-up Foundation of Foshan Graduate School of Innovation, Northeastern University[FSNEU20201016003] ; Scientific Research Project of Foshan Talents[200076622001] ; Scientific Research Project of Foshan Talents[200076622004] ; Open Fund of the State Key Laboratory of Optoelectronic Materials and Technologies (Sun Yat-Sen University)[OEMT-2023-KF-02] ; [52202166] |
WOS研究方向 | Chemistry |
WOS类目 | Chemistry, Physical |
WOS记录号 | WOS:001230756900001 |
出版者 | WILEY-V C H VERLAG GMBH |
引用统计 | |
文献类型 | 期刊论文 |
条目标识符 | http://ir.imr.ac.cn/handle/321006/186485 |
专题 | 中国科学院金属研究所 |
通讯作者 | Li, Jing; Yao, Jinlei; Liu, Baodan |
作者单位 | 1.Northeastern Univ, Sch Mat Sci & Engn, 11 Wenhua Rd, Shenyang 110819, Peoples R China 2.Northeastern Univ, Foshan Grad Sch Innovat, 11 Wenhua Rd, Shenyang 110819, Peoples R China 3.Chinese Acad Sci, Inst Met Res, Shenyang Natl Lab Mat Sci, 72 Wenhua Rd, Shenyang 110016, Peoples R China 4.Suzhou Univ Sci & Technol, Sch Phys Sci & Technol, Jiangsu Key Lab Micro & Nano Heat Fluid Flow Techn, Suzhou 215009, Peoples R China |
推荐引用方式 GB/T 7714 | Hua, Zhe,Yang, Liu,Li, Jing,et al. Mesoporous Pt/N-TiO2/Ti Photocatalytic Plate for Highly Efficient Hydrogen Production[J]. CHEMCATCHEM,2024:10. |
APA | Hua, Zhe.,Yang, Liu.,Li, Jing.,Wang, Junchao.,Chen, Lixin.,...&Liu, Baodan.(2024).Mesoporous Pt/N-TiO2/Ti Photocatalytic Plate for Highly Efficient Hydrogen Production.CHEMCATCHEM,10. |
MLA | Hua, Zhe,et al."Mesoporous Pt/N-TiO2/Ti Photocatalytic Plate for Highly Efficient Hydrogen Production".CHEMCATCHEM (2024):10. |
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