Liquid metal-embraced photoactive films for artificial photosynthesis

doi:10.1038/s41467-024-46073-6

IMR OpenIR

	Liquid metal-embraced photoactive films for artificial photosynthesis
	Zhen, Chao 1; Chen, Xiangtao 2; Chen, Ruotian 3; Fan, Fengtao 3; Xu, Xiaoxiang 4; Kang, Yuyang 1; Guo, Jingdong 1; Wang, Lianzhou 5,6; Lu, Gao Qing (Max)7; Domen, Kazunari 8,9; Cheng, Hui-Ming 1,10; Liu, Gang 1,11
通讯作者	Liu, Gang(gangliu@imr.ac.cn)
	2024-02-23
发表期刊	NATURE COMMUNICATIONS
卷号	15 期号:1 页码:13
摘要	The practical applications of solar-driven water splitting pivot on significant advances that enable scalable production of robust photoactive films. Here, we propose a proof-of-concept for fabricating robust photoactive films by a particle-implanting technique (PiP) which embeds semiconductor photoabsorbers in the liquid metal. The strong semiconductor/metal interaction enables resulting films efficient collection of photogenerated charges and superior photoactivity. A photoanode of liquid-metal embraced BiVO4 can stably operate over 120 h and retain similar to 70% of activity when scaled from 1 to 64 cm(2). Furthermore, a Z-scheme photocatalyst film of liquid-metal embraced BiVO4 and Rh-doped SrTiO3 particles can drive overall water splitting under visible light, delivering an activity 2.9 times higher than that of the control film with gold support and a 110 h stability. These results demonstrate the advantages of the PiP technique in constructing robust and efficient photoactive films for artificial photosynthesis.
资助者	National Natural Science Foundation of China (National Science Foundation of China) ; National Key R&D Program of China ; National Natural Science Foundation of China ; CAS Projects for Young Scientists in Basic Research ; Youth Innovation Promotion Association of the Chinese Academy of Sciences ; New Cornerstone Science Foundation through the XPLORER PRIZE
DOI	10.1038/s41467-024-46073-6
收录类别	SCI
语种	英语
资助项目	National Natural Science Foundation of China (National Science Foundation of China)[2021YFA1500800] ; National Key R&D Program of China[51825204] ; National Key R&D Program of China[52072377] ; National Key R&D Program of China[51972312] ; National Key R&D Program of China[52188101] ; National Natural Science Foundation of China[YSBR-004] ; CAS Projects for Young Scientists in Basic Research[2020192] ; Youth Innovation Promotion Association of the Chinese Academy of Sciences ; New Cornerstone Science Foundation through the XPLORER PRIZE
WOS研究方向	Science & Technology - Other Topics
WOS类目	Multidisciplinary Sciences
WOS记录号	WOS:001176993700027
出版者	NATURE PORTFOLIO
引用统计	被引频次：14[WOS] [WOS记录] [WOS相关记录]
文献类型	期刊论文
条目标识符	http://ir.imr.ac.cn/handle/321006/185334
专题	中国科学院金属研究所
通讯作者	Liu, Gang
作者单位	1.Chinese Acad Sci, Inst Met Res, Shenyang Natl Lab Mat Sci, 72 Wenhua Rd, Shenyang 110016, Peoples R China 2.Northeastern Univ, Key Lab Anisotropy & Texture Mat, Minist Educ, Shenyang 110819, Liaoning, Peoples R China 3.Chinese Acad Sci, Dalian Inst Chem Phys, State Key Lab Catalysis, Dalian Natl Lab Clean Energy,iChEM, Dalian, Peoples R China 4.Tongji Univ, Sch Chem Sci & Engn, Shanghai 200092, Peoples R China 5.Univ Queensland, Nanomat Ctr, Sch Chem Engn, Brisbane, Qld 4072, Australia 6.Univ Queensland, AIBN, Brisbane, Qld 4072, Australia 7.Univ Surrey, Guildford GU2 7XH, England 8.Shinshu Univ, Res Initiat Supramat, Nagano, Japan 9.Univ Tokyo, Off Univ Prof, Tokyo, Japan 10.Chinese Acad Sci, Shenzhen Inst Adv Technol, 1068 Xueyuan Blvd, Shenzhen 518055, Peoples R China 11.Univ Sci & Technol China, Sch Mat Sci & Engn, 72 Wenhua Rd, Shenyang 110016, Peoples R China
推荐引用方式 GB/T 7714	Zhen, Chao,Chen, Xiangtao,Chen, Ruotian,et al. Liquid metal-embraced photoactive films for artificial photosynthesis[J]. NATURE COMMUNICATIONS,2024,15(1):13.
APA	Zhen, Chao.,Chen, Xiangtao.,Chen, Ruotian.,Fan, Fengtao.,Xu, Xiaoxiang.,...&Liu, Gang.(2024).Liquid metal-embraced photoactive films for artificial photosynthesis.NATURE COMMUNICATIONS,15(1),13.
MLA	Zhen, Chao,et al."Liquid metal-embraced photoactive films for artificial photosynthesis".NATURE COMMUNICATIONS 15.1(2024):13.