IMR OpenIR
Fe-26Cr-IMO不锈钢腐蚀疲劳行为与机制
颜晓明
学位类型硕士
导师王中光
1990
学位授予单位中国科学院金属研究所
学位授予地点中国科学院金属研究所
摘要本文采用塑性应变幅控制方式研究了Fe-26Cr-1 Mo超纯铁素体不锈钢的空气疲劳和腐蚀疲劳行为。在空气中的疲劳实验结果显示,其循环硬化现象随着应变幅的增加而愈加明显。在高应变速率和高应变幅下,裂纹主要从晶界萌生;而在低应变幅和低应变速率下,裂纹主要在晶内滑移带产生。这些行为均可从位错的热激活理论出发给予合理的解释。对于腐蚀疲劳,为实现应变控制和腐蚀电流测量,发展了一套新颖的腐蚀疲劳实验系统。实验主要在钝化电位区间进行。在1M H_2SO_4中的腐蚀疲劳实验展示了一些有趣的新现象:1)弹性拉应变使印化电流减小,使得在以先拉开始的疲劳实验中出现电流“小凹”,而弹性压应变却无此表现;2)在循环硬化达到饱和时,瞬态电流开始衰减;3)对于较高的塑性应变幅,拉、压最大时均有瞬态电流峰出现,而在低应变幅下,一个应变周期只对应一个电流峰。在1M NaCl中,瞬态电流行为与1M H_2SO_4中的差异甚大。一个应变周期只对应一个变峰,腐蚀电流随着应变循环的进行持续上升,但电流峰高却恒定不变。变频和变幅实验均显示电流幅高与应变速率成正比。本文认为,对于1M H_2SO_4中的腐蚀疲劳行为可按钝化膜破裂模型来理解,而对于1M H_2SO_4中的腐蚀疲劳,膜破裂模型并不有效。提出了“膜畸变”之说以试图解释之。对于拉、压弹性应变对钝化电流的影响,认为泊松效应使固态晶体膜变薄,导致介电常数增加是最重要的原因。1M H_2SO_4中的电流下降被归因为在疲劳初期的改善。
其他摘要Fatigue experiments have been conducted with high purity ferritic stainless steel Fe-26Cr-1Mo in air and corrosive solutions under plastic strain control. The results in air show that the cyclic hardening becomes more and more pronounced with increasing plastic strain amplitude and strain rate, Fatigue cracks usually initiate along the persistent slip bands in the cases of low strain amplitude and low cyclic strain rate, but cracks nucleant at the grain boundaries while the strain amplitude and strain rate are higher. Such behaviors can be explained according t the thermal activation theory of dislocations. A sensitive apparatus was specially developed for carrying out corrosion fatigue experiments under plastic strain control. The corrosion transient current could be accurately measured with this device. All corrosion fatigue experiments were performed within the potential range of passivity. Fatigue in 1M H_2SO_4 solution shows several interesting points. Firstly, a bump of current was found in the first half cycle when the tests started with tension. However, such behavior did not occur in the tests starting with compression. Secondly, at the strain amplitude above 2.8 * 10~(-3), there are two transient current peaks in one strain cycle. However, there is only one peak in one strain cycle when the strain amplitude is below 1.4 * 10~(-3).Thirdly, corrosion current began to decrease as soon as the cyclic handening reached saturation. Corrosion current behavior during fatigue in 1M Nacl solution was greatly different from that in 1M H_2SO_4 solution. Here, in one strain cycle, only one current peak could be found and the corrosion current increases continuously with cycling but the current amplitude remains unchanged. It was concluded that the current behavior in corrosion fatigue in 1M H_2SO_4 could be attributed to the repeated rupture of the passive film. However, in 1M Nacl solution, the corrosion fatigue behavior can not be interpreted by the model of film rupture. A model of distortion of passive film was proposed. It was suggested that the bump of current was caused by the increase of dielectric constant, which resulted from thinning solid passive film due to Poisson's effect. The decay of corrosion current at cyclic saturation regime was considered to be caused by the improvement of oxide film in quality during corrosion fatigue.
页数74
语种中文
文献类型学位论文
条目标识符http://ir.imr.ac.cn/handle/321006/17453
专题中国科学院金属研究所
推荐引用方式
GB/T 7714
颜晓明. Fe-26Cr-IMO不锈钢腐蚀疲劳行为与机制[D]. 中国科学院金属研究所. 中国科学院金属研究所,1990.
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