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含氧化铈的镍铬复合镀渗铝涂层及其高温腐蚀
敬安晋
学位类型硕士
导师李铁藩
1990
学位授予单位中国科学院金属腐蚀与防护研究所
学位授予地点中国科学院金属腐蚀与防护研究所
摘要本文采用复合电镀和分层电镀的方法在M_(38)高温合金上电镀含Cr量和CeO_2不相同的Ni + CeO_2/Cr/Ni + CeO_2复合镀层,分别经真空扩散处理后和不经真空扩散处理再一起进行高活度渗Al制成了βNi(Cr)Al + CeO_2系列复合涂层。研究了βNi(Cr)Al + CeO_2系列涂层和βNi(Cr)Al及M_(38)渗Al涂层1100 ℃高温静态空气中氧化及氧化皮剥落特性,用不连续称重法测了各种涂层的动力学曲线。以及这些涂层在900 ℃高温下,100小时的混合盐(75%NaSO_4 + 25%NaCl)热腐蚀。使用电子探针分析截面元素分布,用X-射线分析氧化及热腐蚀后的产物,用金相方法观察显微组织结构。实验结果表明:含CeO_2的涂层抗氧化作用效果远低于不含CeO_2的涂层;在含CeO_2的所有涂层中,含CeO_2少的抗氧化作用效果优于含CeO_2多的抗氧化作用效果;渗铝前进行真空扩散处理的涂层抗氧化性优于不经真空扩散处理的涂层抗氧化性;含Cr量高的涂层抗氧化作用效果优于含Cr量低的涂层抗氧化作用效果;CeO_2的加入能明显地改善涂层氧化膜粘附性,含CeO_2的涂层抗热腐蚀作用好于不含CeO_2的涂层,含CeO_2多的涂层好于含CeO_2少的涂层抗热腐蚀作用效果。分析和讨论了所得的实验结果;探讨了CeO_2的作用机理。
其他摘要By means of multistep techniques a serial of composite coatings of Cr and CeO_2 Containing nickel aluminide Ni(Cr)Al+CeO_2 for superalloy M_(38) have been developed. Firstly, the sandwich platings of Ni + CeO_2/Cr/Ni + CeO_2 with desired Cr and CeO_2 contents were successively electro deposited using conrentronal plating baths. Secondly, the plated samples with or without a post heat treatment were then aluminized through a high activity pack cementation process. In order to compare the oxidation performance of the new developed composite coatings of Ni(Cr)Al + CeO_2 with the coatings of Ni(Cr)Al without CeO_2, NiAl + CeO_2 without Cr and the simple aluminide of M_(38), they have been tested in air at 1100 ℃ for 200 hrs, and their hot corrosion behavior has also been examined by immersing the samples in crucibles with melten 75Na_2SO_4 + 25NaCl salt in air at 900 ℃ for 100 hrs. The morphology and phase constituents of oxidation and hot corrosion products are examined by optical metalloyraphy scanny electron microscopy, electroprobe microanalysis and X-ray diffraction. It follows that all the Ni(Cr)Al + CeO_2 composite coatings show better oxidation resistance than that of Ni(Cr)Al and simple alumimide coatings, However amount the CeO_2 coating Ni(Cr)Al coatings; the one with less CeO_2 content shows lower oxidation rate, it is also observed that the decrease in oxidation rate due to the addition of CeO_2 is primarily associated with improvement in scale adhesion. Higher Cr content and a heat treatment between the plating and the aluminizing steps are separatly beneficial to the oxidation resistance of the Ni(Cr)Al + CeO_2 coatings. The hot corrosion behavior of the Ni(Cr)Al type coatings is improved by the addition of CeO_2. The higher CeO_2 content shows the better corrosion reisistance of the coating. The matter maybe ascribed to the trapping effect for s by the cerium oxide. The degradation process of the coatings is discussed as well.
页数47
语种中文
文献类型学位论文
条目标识符http://ir.imr.ac.cn/handle/321006/17436
专题中国科学院金属研究所
推荐引用方式
GB/T 7714
敬安晋. 含氧化铈的镍铬复合镀渗铝涂层及其高温腐蚀[D]. 中国科学院金属腐蚀与防护研究所. 中国科学院金属腐蚀与防护研究所,1990.
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