Nature-Inspired Nacre-Like Composites Combining Human Tooth-Matching Elasticity and Hardness with Exceptional Damage Tolerance

doi:10.1002/adma.201904603

IMR OpenIR

	Nature-Inspired Nacre-Like Composites Combining Human Tooth-Matching Elasticity and Hardness with Exceptional Damage Tolerance
	Tan, Guoqi 1,2; Zhang, Jian 1; Zheng, Long 3; Jiao, Da 1; Liu, Zengqian 1,2; Zhang, Zhefeng 2; Ritchie, Robert O.1,4
通讯作者	Liu, Zengqian(zengqianliu@imr.ac.cn) ; Zhang, Zhefeng(zhfzhang@imr.ac.cn) ; Ritchie, Robert O.(roritchie@lbl.gov)
	2019-11-12
发表期刊	ADVANCED MATERIALS
ISSN	0935-9648
页码	9
摘要	Making replacements for the human body similar to natural tissue offers significant advantages but remains a key challenge. This is pertinent for synthetic dental materials, which rarely reproduce the actual properties of human teeth and generally demonstrate relatively poor damage tolerance. Here new bioinspired ceramic-polymer composites with nacre-mimetic lamellar and brick-and-mortar architectures are reported, which resemble, respectively, human dentin and enamel in hardness, stiffness, and strength and exhibit exceptional fracture toughness. These composites are additionally distinguished by outstanding machinability, energy-dissipating capability under cyclic loading, and diminished abrasion to antagonist teeth. The underlying design principles and toughening mechanisms of these materials are elucidated in terms of their distinct architectures. It is demonstrated that these composites are promising candidates for dental applications, such as new-generation tooth replacements. Finally, it is believed that this notion of bioinspired design of new materials with unprecedented biologically comparable properties can be extended to a wide range of material systems for improved mechanical performance.
关键词	bioinspiration composites elasticity fracture toughness teeth
资助者	National Natural Science Foundation of China ; U.S. Air Force Office of Scientific Research, under MURI grant
DOI	10.1002/adma.201904603
收录类别	SCI
语种	英语
资助项目	National Natural Science Foundation of China[51871216] ; National Natural Science Foundation of China[51501190] ; U.S. Air Force Office of Scientific Research, under MURI grant[AFSOR-FA9550-15-1-0009]
WOS研究方向	Chemistry ; Science & Technology - Other Topics ; Materials Science ; Physics
WOS类目	Chemistry, Multidisciplinary ; Chemistry, Physical ; Nanoscience & Nanotechnology ; Materials Science, Multidisciplinary ; Physics, Applied ; Physics, Condensed Matter
WOS记录号	WOS:000496433700001
出版者	WILEY-V C H VERLAG GMBH
引用统计	被引频次：115[WOS] [WOS记录] [WOS相关记录]
文献类型	期刊论文
条目标识符	http://ir.imr.ac.cn/handle/321006/136866
专题	中国科学院金属研究所
通讯作者	Liu, Zengqian; Zhang, Zhefeng; Ritchie, Robert O.
作者单位	1.Chinese Acad Sci, Lab Fatigue & Fracture Mat, Inst Met Res, Shenyang 110016, Liaoning, Peoples R China 2.Univ Sci & Technol China, Sch Mat Sci & Engn, Hefei 230026, Anhui, Peoples R China 3.Jilin Univ, Key Lab Bion Engn, Minist Educ, Coll Biol & Agr Engn, Changchun 130022, Jilin, Peoples R China 4.Univ Calif Berkeley, Dept Mat Sci & Engn, Berkeley, CA 94720 USA
推荐引用方式 GB/T 7714	Tan, Guoqi,Zhang, Jian,Zheng, Long,et al. Nature-Inspired Nacre-Like Composites Combining Human Tooth-Matching Elasticity and Hardness with Exceptional Damage Tolerance[J]. ADVANCED MATERIALS,2019:9.
APA	Tan, Guoqi.,Zhang, Jian.,Zheng, Long.,Jiao, Da.,Liu, Zengqian.,...&Ritchie, Robert O..(2019).Nature-Inspired Nacre-Like Composites Combining Human Tooth-Matching Elasticity and Hardness with Exceptional Damage Tolerance.ADVANCED MATERIALS,9.
MLA	Tan, Guoqi,et al."Nature-Inspired Nacre-Like Composites Combining Human Tooth-Matching Elasticity and Hardness with Exceptional Damage Tolerance".ADVANCED MATERIALS (2019):9.